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ALS Work Using Spectroscopy

These techniques are used to study the energies of particles that are emitted or absorbed by samples that are exposed to the light-source beam and are commonly used to determine the characteristics of chemical bonding and electron motion.

 

Understanding Electronic Structure in MXenes, One Atomic Layer at a Time

MXenes are 2D materials that can host a rich array of distinct chemical compositions that can be tuned for a broad range of applications, from energy storage to water purification. Site-specific x-ray absorption spectroscopy helped identify the unique roles of surface and subsurface transition-metal atoms in Ti-based MXenes. Read more »

A Probe of Light-Harvesting Efficiency at the Nanoscale

Using time-resolved experiments at the ALS, researchers found a way to count electrons moving back and forth across a model interface for photoelectrochemical cells. The findings provide real-time, nanoscale insight into the efficiency of nanomaterial catalysts that help turn sunlight and water into fuel through artificial photosynthesis. Read more »PPT-icon-35 PDF-icon-35

The Flat Band in Magic-Angle Graphene Visualized

Researchers visualized flat band structures associated with exotic electronic phases in stacked graphene layers offset from each other by a “magic angle.” The work corroborates theoretical predictions and has significant implications for phenomena of technological and fundamental interest, such as topological phases and superconductivity. Read more »PPT-icon-35 PDF-icon-35

Site-dependent selectivity in oxidation reactions on single Pt nanoparticles

Heterogeneous catalysis is a surface-controlled phenomenon in which different surface sites often show variations in reactivity, posing a major complication for the chemical industry. Here, site-dependent selectivity in oxidation reactions on Pt nanoparticles was identified by conducting IR nanospectroscopy measurements while using allyl-functionalized N-heterocyclic carbenes (allyl-NHCs) as probe molecules. Read more »

2D Electronics Get an Atomic Tuneup

Researchers demonstrated a promising avenue for controlling atomic ordering in semiconductor alloys by engineering frustrated interactions in a 2D transition metal dichalcogenide (TMD). The work could lead to improved semiconductor performance for next-generation electronics such as optoelectronics, thermoelectrics, and sensors. Read more »

How Water Promotes Catalysis of Methane to Methanol

Researchers unraveled how water helps catalyze the conversion of methane, the main component of natural gas, into methanol, a liquid fuel. The work supports the efficient production of methanol and other useful chemicals and could help reduce the amount of greenhouse gases released by the flaring and venting of methane. Read more »PPT-icon-35 PDF-icon-35

2020 Shirley Award to Honor Miquel Salmeron

By taking surface studies from ultrahigh vacuum to near-ambient pressure, Miquel Salmeron’s work at the ALS has had deep impact on a broad range of scientific questions, revealing the chemical, electronic, and mechanical properties of surfaces and interfaces on the nanometer (and often atomic) scale. Read more »

Scientists Dive Deep Into Hidden World of Quantum States

Researchers discovered two unique electronic properties—a Van Hove singularity and Fermi surface topology—at the interface between atomically thin oxide materials. The results suggest that the system is an ideal platform for investigating how to control superconductivity at the atomic scale in 2D materials. Read more »